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Gmail is the Google approach to email and chat. Practically unlimited free online storage allows you to collect all your messages, and Gmail's simple but very smart interface lets you find them precisely and see them in context without effort.
AIM Mail, AOL's free web-based email service, shines with unlimited online storage, very good spam protection and a rich, easy to use interface.
GMX Mail is a reliable email service filtered well of spam and viruses whose 5 GB of online storage you can use not only through a rich web interface but also via POP or IMAP from a desktop email program.
Yahoo! Mail is your ubiquitous email program on the web with unlimited storage and RSS news feeds, SMS texting and instant messaging to boot.
Zenbe Personal organizes your emails and attachments (from Zenbe and existing POP accounts) with labels and search — and integrates calendar, to-do list, twitter and Facebook updates, too.
Gawab.com is a speedy, stable and very usable free email service with 10 GB online space, POP and IMAP access as well as many a web-based goodie.
Inbox.com not only gives you 5 GB to store your mail online but also a highly polished, fast and functional way to access it via either the web (including speedy search, free-form labels and reading mail by conversation) or through POP in your email program.
FastMail is a great free email service with IMAP access, useful features, and a stellar web interface.